%0 Journal Article %T Dimensional crossover in the quasi-one-dimensional superconductor Tl2Mo6Se6 %+ Nanyang Technological University [Singapour] %+ Université Libanaise %+ Institut des Sciences Chimiques de Rennes (ISCR) %+ Los Alamos National Laboratory (LANL) %A Mitra, S. %A Petrovic, A. P. %A Salloum, D. %A Gougeon, Patrick %A Potel, M. %A Zhu, Jian-Xin %A Panagopoulos, C. %A Chia, Elbert E. M. %Z Singapore Ministry of Education (MOE) Tier 1 grant [RG13/12] %Z Singapore Ministry of Education (MOE) Tier 2 grant [MOE2015-T2-2-065] %Z Singapore National Research Foundation (NRF) Investigatorship [NRF-NRFI2015-04] %Z U.S. DOE Office of Basic Energy Sciences (BES) Core Program E3B7 %Z Center for Integrated Nanotechnologies, a U.S. DOE BES user facility %< avec comité de lecture %@ 2469-9950 %J Physical Review B %I American Physical Society %V 98 %N 5 %P 054507 %8 2018 %D 2018 %Z 1710.00292 %R 10.1103/PhysRevB.98.054507 %Z Chemical SciencesJournal articles %X We present magnetic penetration depth and electrical transport data in single crystals of quasi-one-dimensional (q1D) Tl2Mo6Se6, which reveal a 1D -> 3D superconducting dimensional crossover. The c-axis penetration depth shows the onset of superconducting fluctuations below T-1D(ons) = 6.7 K, whereas signatures of superconductivity in the ab-plane penetration depth (a uniquely sensitive probe of the transverse phase stiffness) only emerge below T-3D(ons) = 4.9 K. An anomalously low superfluid density persists down to similar to 3 K before rising steeply, in agreement with a theoretical model for crossovers in q1D superconductors. Our data analysis suggests that a sequence of pairing and phase fluctuation regimes controls the unusually broad superconducting transition. In particular, the electrical resistivity below T-3D(ons) is quantitatively consistent with the establishment of phase coherence through gradual binding of Josephson vortex strings to form 3D loops. This dimensional crossover within the superconducting state occurs despite the relatively large transverse hopping predicted from the band structure. Our results have important consequences for the low-temperature normal state in Tl2Mo6Se6 and similar q1D metals, which may retain one-dimensional behavior to lower temperatures than expected from theory. %G English %L hal-01879777 %U https://univ-rennes.hal.science/hal-01879777 %~ UNIV-RENNES1 %~ CNRS %~ INSA-RENNES %~ ENSC-RENNES %~ ISCR %~ ISCR-CSM %~ STATS-UR1 %~ UR1-SPM %~ INC-CNRS %~ UR1-UFR-SPM %~ UR1-HAL %~ UR1-SDLM %~ TEST-UR-CSS %~ UNIV-RENNES %~ INSA-GROUPE %~ TEST-HALCNRS %~ UR1-MMS %~ TEST2-HALCNRS